Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction

Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction

While the degradation of materials during usage is crucial in understanding their performance, it is challenging to understand the corrosion processes. Here, authors find copper nanoparticles to undergo an unusual potential-driven nanoclustering degradation pathway during carbon dioxide reduction.

Bibliographic Details
Main Authors: Jianfeng Huang, Nicolas Hörmann, Emad Oveisi, Anna Loiudice, Gian Luca De Gregorio, Oliviero Andreussi, Nicola Marzari, Raffaella Buonsanti
Format: Article
Language:English
Published: Nature Publishing Group 2018-08-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-018-05544-3
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spelling doaj-073f1c572a7149dcba0c35c3ae7fd45e2021-05-11T09:48:45ZengNature Publishing GroupNature Communications2041-17232018-08-01911910.1038/s41467-018-05544-3Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reductionJianfeng Huang0Nicolas Hörmann1Emad Oveisi2Anna Loiudice3Gian Luca De Gregorio4Oliviero Andreussi5Nicola Marzari6Raffaella Buonsanti7Laboratory of Nanochemistry for Energy (LNCE), Department of Chemical Sciences and Engineering, École Polytechnique Fédérale de LausanneTheory and Simulation of Materials (THEOS), and National Centre for Computational Design and Discovery of Novel Materials (MARVEL), École Polytechnique Fédérale de LausanneInterdisciplinary Centre for Electron Microscopy (CIME), École Polytechnique Fédérale de LausanneLaboratory of Nanochemistry for Energy (LNCE), Department of Chemical Sciences and Engineering, École Polytechnique Fédérale de LausanneLaboratory of Nanochemistry for Energy (LNCE), Department of Chemical Sciences and Engineering, École Polytechnique Fédérale de LausanneTheory and Simulation of Materials (THEOS), and National Centre for Computational Design and Discovery of Novel Materials (MARVEL), École Polytechnique Fédérale de LausanneTheory and Simulation of Materials (THEOS), and National Centre for Computational Design and Discovery of Novel Materials (MARVEL), École Polytechnique Fédérale de LausanneLaboratory of Nanochemistry for Energy (LNCE), Department of Chemical Sciences and Engineering, École Polytechnique Fédérale de LausanneWhile the degradation of materials during usage is crucial in understanding their performance, it is challenging to understand the corrosion processes. Here, authors find copper nanoparticles to undergo an unusual potential-driven nanoclustering degradation pathway during carbon dioxide reduction.https://doi.org/10.1038/s41467-018-05544-3
collection DOAJ
language English
format Article
sources DOAJ
author Jianfeng Huang
Nicolas Hörmann
Emad Oveisi
Anna Loiudice
Gian Luca De Gregorio
Oliviero Andreussi
Nicola Marzari
Raffaella Buonsanti
spellingShingle Jianfeng Huang
Nicolas Hörmann
Emad Oveisi
Anna Loiudice
Gian Luca De Gregorio
Oliviero Andreussi
Nicola Marzari
Raffaella Buonsanti
Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction
Nature Communications
author_facet Jianfeng Huang
Nicolas Hörmann
Emad Oveisi
Anna Loiudice
Gian Luca De Gregorio
Oliviero Andreussi
Nicola Marzari
Raffaella Buonsanti
author_sort Jianfeng Huang
title Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction
title_short Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction
title_full Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction
title_fullStr Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction
title_full_unstemmed Potential-induced nanoclustering of metallic catalysts during electrochemical CO2 reduction
title_sort potential-induced nanoclustering of metallic catalysts during electrochemical co2 reduction
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2018-08-01
description While the degradation of materials during usage is crucial in understanding their performance, it is challenging to understand the corrosion processes. Here, authors find copper nanoparticles to undergo an unusual potential-driven nanoclustering degradation pathway during carbon dioxide reduction.
url https://doi.org/10.1038/s41467-018-05544-3
work_keys_str_mv AT jianfenghuang potentialinducednanoclusteringofmetalliccatalystsduringelectrochemicalco2reduction
AT nicolashormann potentialinducednanoclusteringofmetalliccatalystsduringelectrochemicalco2reduction
AT emadoveisi potentialinducednanoclusteringofmetalliccatalystsduringelectrochemicalco2reduction
AT annaloiudice potentialinducednanoclusteringofmetalliccatalystsduringelectrochemicalco2reduction
AT gianlucadegregorio potentialinducednanoclusteringofmetalliccatalystsduringelectrochemicalco2reduction
AT olivieroandreussi potentialinducednanoclusteringofmetalliccatalystsduringelectrochemicalco2reduction
AT nicolamarzari potentialinducednanoclusteringofmetalliccatalystsduringelectrochemicalco2reduction
AT raffaellabuonsanti potentialinducednanoclusteringofmetalliccatalystsduringelectrochemicalco2reduction
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