Flexible perovskite based X-ray detectors for dose monitoring in medical imaging applications
Organometallic halide perovskite materials are attracting considerable interest for high performance photovoltaic and photodetector applications due to their exceptional opto-electronic properties and easy processing capability. The high atomic numbers (Z) of their constituents also make these mater...
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doaj-065fa81f348d4d8caa1cba5f85cc14122020-11-25T00:32:05ZengElsevierPhysics in Medicine2352-45102018-06-0152023Flexible perovskite based X-ray detectors for dose monitoring in medical imaging applicationsHardeep Singh Gill0Bassem Elshahat1Akshay Kokil2Lian Li3Ravi Mosurkal4Piotr Zygmanski5Erno Sajo6Jayant Kumar7Center for Advanced Materials, University of Massachusetts Lowell, Lowell, MA 01854, USA; Department of Physics and Applied Physics, University of Massachusetts Lowell, Lowell, MA 01854, USADepartment of Physics and Applied Physics, University of Massachusetts Lowell, Lowell, MA 01854, USA; Department of Medical Imaging, Royal Jubille Hospital, Vancouver Island Authority, Victoria, BC V8R 1J8, CanadaCenter for Advanced Materials, University of Massachusetts Lowell, Lowell, MA 01854, USABio-science Team, US Army Natick Soldier Research, Development & Engineering Center, Natick, MA 01760, USABio-science Team, US Army Natick Soldier Research, Development & Engineering Center, Natick, MA 01760, USADepartment of Radiation Oncology, Brigham and Women's Hospital & Dana Faber Cancer Institute, Harvard Medical School, Boston, MA 02115, USADepartment of Physics and Applied Physics, University of Massachusetts Lowell, Lowell, MA 01854, USACenter for Advanced Materials, University of Massachusetts Lowell, Lowell, MA 01854, USA; Department of Physics and Applied Physics, University of Massachusetts Lowell, Lowell, MA 01854, USA; Corresponding author. Center for Advanced Materials, University of Massachusetts Lowell, Lowell, MA 01854, USA.Organometallic halide perovskite materials are attracting considerable interest for high performance photovoltaic and photodetector applications due to their exceptional opto-electronic properties and easy processing capability. The high atomic numbers (Z) of their constituents also make these materials suitable for X-ray detection. Here we report on the direct detection of X-ray induced photocurrents in flexible organolead halide perovskite based detectors. The electrical response of the detectors was found to be linear with the radiation dosage. These perovskite based radiation detectors were about 550% more sensitive than commonly used amorphous silicon solar devices. The high sensitivity to the X-rays could be attributed to the high Z constituents and large charge carrier mobility. Our results indicate that the perovskite materials are promising candidates for direct X-ray detectors. Keywords: X-ray detectors, Dosimeterhttp://www.sciencedirect.com/science/article/pii/S2352451018300088 |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Hardeep Singh Gill Bassem Elshahat Akshay Kokil Lian Li Ravi Mosurkal Piotr Zygmanski Erno Sajo Jayant Kumar |
spellingShingle |
Hardeep Singh Gill Bassem Elshahat Akshay Kokil Lian Li Ravi Mosurkal Piotr Zygmanski Erno Sajo Jayant Kumar Flexible perovskite based X-ray detectors for dose monitoring in medical imaging applications Physics in Medicine |
author_facet |
Hardeep Singh Gill Bassem Elshahat Akshay Kokil Lian Li Ravi Mosurkal Piotr Zygmanski Erno Sajo Jayant Kumar |
author_sort |
Hardeep Singh Gill |
title |
Flexible perovskite based X-ray detectors for dose monitoring in medical imaging applications |
title_short |
Flexible perovskite based X-ray detectors for dose monitoring in medical imaging applications |
title_full |
Flexible perovskite based X-ray detectors for dose monitoring in medical imaging applications |
title_fullStr |
Flexible perovskite based X-ray detectors for dose monitoring in medical imaging applications |
title_full_unstemmed |
Flexible perovskite based X-ray detectors for dose monitoring in medical imaging applications |
title_sort |
flexible perovskite based x-ray detectors for dose monitoring in medical imaging applications |
publisher |
Elsevier |
series |
Physics in Medicine |
issn |
2352-4510 |
publishDate |
2018-06-01 |
description |
Organometallic halide perovskite materials are attracting considerable interest for high performance photovoltaic and photodetector applications due to their exceptional opto-electronic properties and easy processing capability. The high atomic numbers (Z) of their constituents also make these materials suitable for X-ray detection. Here we report on the direct detection of X-ray induced photocurrents in flexible organolead halide perovskite based detectors. The electrical response of the detectors was found to be linear with the radiation dosage. These perovskite based radiation detectors were about 550% more sensitive than commonly used amorphous silicon solar devices. The high sensitivity to the X-rays could be attributed to the high Z constituents and large charge carrier mobility. Our results indicate that the perovskite materials are promising candidates for direct X-ray detectors. Keywords: X-ray detectors, Dosimeter |
url |
http://www.sciencedirect.com/science/article/pii/S2352451018300088 |
work_keys_str_mv |
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